 If you liked
Darker than Black: Kuro no Keiyakusha
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 ...then you might like
Guilty Crown
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Both series contain sci-fi themes mixed in with action and drama. Additionally, both series have a darker mood as the episodes progresses. There is also a bit of mystery in both series covered up malevolence.
In addition, the main character are accompanied by a girl with supernatural powers and with a similar stoic personality in which the protagonist tries to save.
They both share a similar theme, that people have 'powers' that can be used for both good and bad. The main Protagonists are trying to fix there past and live a better future but keep getting dragged into situations they would rather avoid.
Its not about the characters so much as the abilities. Lee has special abilities as do most of the people around him that was caused by a mysterious event that not many people no about. He is not fighting a rebellion, so much as stopping a national plot, though indirectly.
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Recommended by Mythical_Truth